Tuning Lasers Towards IR

A laser optical pulse enters into the hollow-core fibre filled with nitrogen gas and, along propagation, experiences a spectral broadening towards longer wavelengths. (Source: R: Piccoli, INRS)

Researchers at Institut national de la recherche scienti­fique INRS have discovered a cost-effective way to tune the spectrum of a laser to the infrared, a band of great interest for many laser appli­cations. They colla­borated with Austrian and Russian research teams to develop this innovation, which is now the subject of a patent appli­cation.

In this field of study, many laser applications have a decisive advantage if the laser wavelength is located and possibly tunable in the infrared region. However, this is still hardly the case with current ultrafast laser techno­logies, and scientists need to explore various nonlinear processes to shift the emission wavelength. In particular, the Optical Para­metric Amplifier (OPA) has so far been the only well-esta­blished tool to reach this infrared window. Although OPA systems offer a broad range of tunability, they are complex, often made of multiples stages, and quite expensive.

The team of Luca Razzari, in colla­boration with Roberto Moran­dotti, has demons­trated that large wavelength tunability can also be achieved with a simple and much less expensive system: a hollow-core (capillary) fiber filled with nitrogen. In addition, this approach readily delivers optical pulses shorter than those of the input laser and with high spatial quality. The researchers also had the benefit of INRS expertise in this field, since the special system to stretch and hold such fibers is marketed by the startup few-cycle.

Usually, hollow-core fibers are filled with a monatomic gas such as argon in order to symme­trically broaden the spectrum of the laser and then recompress it into a much shorter optical pulse. The research team disco­vered that by using a molecular gas such as nitrogen, spectral broadening was still possible, but in an unexpected manner. “Rather than spreading symmetrically, the spectrum was impres­sively shifted toward less energetic infrared wavelengths. This frequency shift is the result of the nonlinear response asso­ciated with the rotation of the gas molecules and, as such, it can be easily controlled by varying the gas pressure (i.e., the number of molecules) in the fiber,” explains Riccardo Piccoli, who led the experi­ments in Razzari’s team.

Once the beam is broadened toward the infrared, the researchers filter the output spectrum to keep only the band of interest. With this approach, energy is transferred into the near-infrared spectral range (with effi­ciency comparable to that of OPAs) in a pulse three times shorter than the input, without any complex apparatus or addi­tional pulse post-compression system. To complete the research, the INRS scientists joined with Austrian and Russian colleagues. “We pooled our expertise after discovering at a conference how similar the phenomena our two groups had observed were,” says Razzari.

The team of researchers based in Vienna headed by Andrius Baltuska and Paolo A. Carpeggiani had a comple­mentary strategy to that of INRS. They also used a nitrogen-filled hollow-core fiber, but rather than filtering the spectrum, they compressed it in time with mirrors capable of adjusting the phase of the broadened pulse. “In this case, the overall shift in the infrared was less extreme, but the final pulse was much shorter and more intense, perfectly suited to atto­second and strong-field physics”, says Carpeggiani.

The Moscow-based team, led by Aleksei Zheltikov, focused on developing a theo­retical model to explain these optical phenomena. By combining these three approaches, the researchers were able to fully understand the complex underlying dynamics as well as achieve not only the extreme red shift using nitrogen, but also efficient pulse compression in the infrared range. The inter­national team believes the method could very well meet the increasing demand for long-wavelength ultrafast sources in laser and strong-field appli­cations, starting with less expensive indus­trial-grade tunable systems based on the emerging ytterbium laser tech­nology. (Source: INRS)

Reference: P. A. Carpeggiani et al.: Extreme Raman red shift: ultrafast multimode nonlinear space-time dynamics, pulse compression, and broadly tunable frequency conversion, Optica 7, 1349 (2020); DOI: 10.1364/OPTICA.397685

Link: Centre Énergie, Matériaux et Télécommunications (EMT), Institut National de la Recherche Scientifique INRS, Varennes, Canada

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