Light-Wave Dynamic Control of Magnetism

Recording of the fast switching of magnetic moments by ultrafast light pulses: The red arrows mark the ordered magnetic moment of a layer stack of nickel and platinum before an ultra-short laser pulse inverts the magnetization of the two layerst. (Source: J.K. Dewhurst)

Electronic properties of materials can be directly influenced via light absorption in under a femtosecond, which is regarded as the limit of the maximum achievable speed of electronic circuits. In contrast, the magnetic moment of matter has only been able to be influenced up to now by a light and magnetism-linked process and roundabout way by means of magnetic fields, which is why magnetic switching takes that much longer and at least several hundred femto­seconds. A consortium of researchers from the Max Planck Institutes for Quantum Optics and for Microstructure Physics, of the Max Born Institute, at the University of Greifswald and Graz University of Technology have only now been able to manipulate the magnetic properties of a ferro­magnetic material on a time scale of electrical field oscil­lations of visible light by means of laser pulses. This influence was able to be accelerated by a factor of 200 and was measured and represented using time-resolved atto­second spectro­scopy.

In attosecond spectro­scopy, magnetic materials are bombarded with ultra-short laser pulses and electronically influenced. “The light flashes set off an intrinsic and usually delaying process in the material. The electronic excitation is translated into a change in magnetic properties,” explains Martin Schultze, who until recently worked at the Max Planck Institute for Quantum Optics in Munich, but who is now professor at the Institute of Experimental Physics at TU Graz. Due to the combi­nation of a ferro­magnet with a non-magnetic metal, the magnetic reaction in the described experiment, however, is brought about as fast as the electronic one. “By means of the special constel­lation, we were optically able to bring about a spatial redistribution of the charge carrier, which resulted in a directly linked change in the magnetic properties,” says Markus Münzen­berg. Together with his team in Greifswald, he developed and produced the special material systems.

Schultze is enthu­siastic about the scale of the success of the research: “Never before has such a fast magnetic phenomenon been observed. Through this, ultrafast magnetism will take on a completely new meaning.” Sangeeta Sharma, researcher at the Max Born Institute in Berlin who predicted the under­lying process using computer models, is impressed: “We are expecting a signi­ficant development boost from this for all appli­cations in which magnetism and electron spin play a role.”

Furthermore, the researchers show in their measure­ments that the observed process runs coherently: this means the quantum mechanical wave nature of the moving charge carriers is preserved. These conditions allow scientists to use individual atoms as information carriers instead of larger units of material or to influence the changing magnetic properties using another speci­fically delayed laser pulse, thus advancing techno­logical minia­turisation. “Regarding new per­spectives, this could lead to similar fantastic developments as in the field of magnetism, such as electronic coherence in quantum computing,” says Schultze hopefully, who now leads a working group focusing on atto­second physics at the Institute of Experimental Physics. (Source: TU Graz)

Reference: F. Siegrist et al.: Light-wave dynamic control of magnetism, Nature, online 26 June 2019; DOI: 10.1038/s41586-019-1333-x

Link: Ultrafast X-Ray Physics, Max-Planck-Institute of Quantum Optics, Garching, Germany

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